Well, Of Course
Actor Nathan Fillion played Captain Mal Reynolds on Firefly and Captain Hammer in Dr. Horrible's Sing-Along Blog. So it's not surprising that people respectfully refer to him as "Captain".
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Captain Tightpants
Which is how he is very commonly referred to, especially on the DVD commentaries.
HA!
I wonder how he'd react to that?
I think you were searching for the 'a' key for 'Mal'